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Step 1
Preheat the oven: Preheat the oven to 300°F.
Step 2
Combine ingredients: Place the meat in a Dutch oven or oven safe pot, and add the beef, peppers, onion, juice from the orange and the remaining orange halves, Cajun seasoning, jalapeños and water. You should have enough water to cover everything in the pot. Bring to a boil over medium-high heat.
Step 3
Cook: Cover the pot and place it in the oven and cook for 3 hours or until the meat falls apart when prodded with a fork. You can also cook this on the stovetop over low heat for 4 hours.
Step 4
Remove the meat: Remove the meat from the pot using a slotted spoon and place it on a baking sheet lined with aluminum foil. Remove everything else from the pot except the liquid using a slotted spoon and discard. Cook the liquid over medium high heat for 20 minutes or until it reduces to about a cup.
Step 5
Shred the meat: Using 2 forks, shred the meat into smaller pieces. Pour the reduced liquid over the shredded meat.
Step 6
Broil meat: Place the baking sheet under the broiler for about 5 to 10 minutes or until browned and crispy. Watch it so that it doesn't burn, each oven is different. Flip the meat and broil for another 5 minutes until brown and crispy.
Step 7
Serve: Serve on tacos or burritos.