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Step 1
Add 5 cups white vinegar, 1.5 cups water and 1 tablespoon salt to a saucepan. Give it a stir, bring to a boil, and remove from heat once boiling.
Step 2
Remove the husks from the tomatillos and give them a good rinse. De-stem the tomatillos and cut them into quarters (or smaller if you want).
Step 3
Add the chopped tomatillos to a quart-sized Mason jar (you could also use two pint-sized Mason jars). We'll also add four peeled, roughly chopped garlic cloves and a single serrano pepper sliced lengthwise.
Step 4
Add 1/2 teaspoon cumin seeds and 1/2 teaspoon black peppercorns to the jar. I give the spices a quick crush in the molcajete to crack the peppercorns but this is optional. (You can also use the bottom of a skillet to accomplish this.)
Step 5
Pour the hot brine mixture over the tomatillos. You should have enough brine to fully submerge the tomatillos.
Step 6
Let the jar cool on the counter for 10-15 minutes, then seal it and store it in the fridge. The tomatillos will be fully pickled in about 24 hours and they'll keep for at least a month in the fridge.